Much later, here's an updated answer without hints. I mostly wanted to see if I could make sense of the details. This proof of almost sure convergence (which implies convergence in probability) complements the supplied proof of convergence in mean square and the direct proof using Chebyshev's inequality.
Proof outline
(1) Show that $Y_n\overset{a.s}{\to}Y$ for some random variable Y.
(2) Show that $\mathbb E Y = \mu := \mathbb E X_1$ and $\mathrm{Var}(Y)=0$
(3) Conclude from this that since (2) implies that $Y = \mu$ a.s., we by (1) have the desired result, namely: $Y_n\overset{a.s}{\to} \mu$.
Proof of 1)
Consider the sum of absolute values, viz.
$$\begin{align}
S_n&:=\sum_{i=1}^n\frac{2i}{n(n+1)}|X_i| \\
& \leq \frac{1}{n}\sum_{i=1}^n|X_i| \overset{a.s,m.s}{\to} \mathbb E|X_i|\leq\sqrt{\mathbb E X_i^2}<\infty
\end{align}$$, where the convergence and inequalities in the last line follows from the strong law of large numbers and the assumption of finite second moment.
This shows that on sets with total probability one, $S_n$ is an increasing and bounded sequence and thus convergent. But $S_n$ is the sum of the absolute values of the terms of the sum $Y_n$, so we thus know that also $Y_n$ converges on these sets. In other words, $Y_n$ is almost surely convergent with limit $Y$, say.
Proof of 2)
We use the following standard result (sometimes called the extended or improved dominated convergence theorem):
A dominated convergence theorem (DCT)
Let $\{Z_n\}$ be a sequence of random variables on some probability space$(\Omega,\mathcal{F},P).$ If $Z_n \overset{a.s}{\to} Z$ and there exist random variables $M_n \overset{a.s}{\to}M$ such that $|Z_n|\leq M_n, \mathbb EM_n<\infty,\forall n$ and $\lim _n \mathbb E M_n = \mathbb E M <\infty$, then $\lim _{n\to \infty} \mathbb E Z_n=\mathbb EZ.$
To obtain the expectation of $Y$, take first $Z_n=Y_n$ and $M_n=\frac{1}{n}\sum_{i=1}^n|X_i|$ in the DCT. We get $\lim _{n\to \infty} \mathbb E Y_n=\lim _{n\to \infty} \mu=\mathbb EY.$
To obtain the variance, set $Z_n=(Y_n-\mu)^2$. We have $Z_n \overset{a.s}{\to}Z:=(Y-\mu)^2$ and also $$|Y_n-\mu|^2\leq (S_n+|\mu|)^2 \leq (\frac{1}{n}\sum_{i=1}^n|X_i|+|\mu|)^2=:M_n.$$
By expanding the square and using the mean square convergence of $\frac{1}{n}\sum_{i=1}^n|X_i|$ it is clear that this $M_n$ satisfies the requirement for applying the DCT. Thus, $$\mathrm{Var}(Y)=\mathbb E (Y-\mu)^2 = \lim_n \mathbb E (Y_n-\mu)^2=\lim_n \mathrm{Var}(Y_n)=0.$$ This finishes the proof.
self-study
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