Both are data adaptive (unlike something like DCT), both can sparsely approximate data (KLT by truncation, dictionary learning by L1 sparsity), yet they different pretty significantly in its implementation.
In (discrete) KLT, PCA + truncation is performed on the expected covariance matrix. In sparse dictionary learning, an alternating optimization scheme is used to approximately solve the problem. In encoding, KLT is just a linear transform but for dictionary learning you solve sparse coding.
What tradeoffs do I make by choosing to use one over the other? Are there types of problems where one is more suitable than the other? Thanks!