As I suggested in comments, in order to see the relationships more clearly, something like the logit and log transforms on mods and sizes respectively at least lets you see more clearly what's happening when "mods" is jammed right up the high end:
This may not be linear, even on this scale; while there's a clear indication that at least that it continues to increase as "sizes" goes up, there's perhaps some suggestion of a kink somewhere around sizes of 70 to 80, after which it increases more slowly, and on this scale it looks almost flat by the largest values of size:
That kind of discussion shouldn't drive your model!
That should come from considerations of what these variables actually are, how they should be related, what might be meaningful for your application.
So:
What are the variables? How are they measured? Why should they be related? Which is the "response", if any? What's the aim of the analysis? What do you need to say about your data and how will you use it?